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Science

Chemists Make First-Ever Ring of Pure Carbon (nature.com) 37

A team of researchers has synthesized the first ring-shaped molecule of pure carbon -- a circle of 18 atoms. Nature reports: The chemists started with a triangular molecule of carbon and oxygen, which they manipulated with electric currents to create the carbon-18 ring. Initial studies of the properties of the molecule, called a cyclocarbon, suggest that it acts as a semiconductor, which could make similar straight carbon chains useful as molecular-scale electronic components.

Chemist Przemyslaw Gawel of the University of Oxford, UK, and his collaborators have now created and imaged the long-sought ring molecule carbon-18. Using standard 'wet' chemistry, his collaborator Lorel Scriven, an Oxford chemist, first synthesized molecules that included four-carbon squares coming off the ring with oxygen atoms attached to squares. The team then sent their samples to IBM laboratories in Zurich, Switzerland, where collaborators put the oxygen -- carbon molecules on a layer of sodium chloride, inside a high-vacuum chamber. They manipulated the rings one at a time with electric currents (using an atomic-force microscope that can also act as a scanning-transmission microscope), to remove the extraneous, oxygen-containing parts. After much trial-and-error, micrograph scans revealed the 18-carbon structure. "I never thought I would see this," says Scriven. Alternating bond types are interesting because they are supposed to give carbon chains and rings the properties of semiconductors. The results suggest that long, straight carbon chains might be semiconductors, too, Gawel says, which could make them useful as components of future molecular-sized transistors.
The paper has been published in the journal Science.
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Chemists Make First-Ever Ring of Pure Carbon

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